Solution Thermodynamics and Kinetics of Metal Complexation with a Hydroxypyridinone Chelator Designed for Thorium-227 Targeted Alpha Therapy

Autor: Deblonde, GJP, Lohrey, TD, Booth, CH, Carter, KP, Parker, BF, Larsen, Å, Smeets, R, Ryan, OB, Cuthbertson, AS, Abergel, RJ

Publikováno v: Inorganic chemistry, vol 57, iss 22
Deblonde, GJP; Lohrey, TD; Booth, CH; Carter, KP; Parker, BF; Larsen, Å; et al.(2018). Solution Thermodynamics and Kinetics of Metal Complexation with a Hydroxypyridinone Chelator Designed for Thorium-227 Targeted Alpha Therapy. Inorganic Chemistry, 57(22), 14337-14346. doi: 10.1021/acs.inorgchem.8b02430. UC Berkeley: Retrieved from: http://www.escholarship.org/uc/item/7nz4j81s

© 2018 American Chemical Society. The solution chemistry of a chelator developed for 227Th targeted alpha therapy was probed. The compound of interest is an octadentate ligand comprising four N-methyl-3-hydroxy-pyridine-2-one metal-binding units, tw

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Investigating subtle 4f vs. 5f coordination differences using kinetically inert Eu(iii), Tb(iii), and Cm(iii) complexes of a coumarin-appended 1,4,7,10-tetraazacyclododecane-1,4,7-triacetate (DO3A) ligand

Autor: Junker, AKR, Deblonde, GJP, Abergel, RJ, Sørensen, TJ

Publikováno v: Junker, AKR; Deblonde, GJP; Abergel, RJ; & Sørensen, TJ. (2018). Investigating subtle 4f vs. 5f coordination differences using kinetically inert Eu(iii), Tb(iii), and Cm(iii) complexes of a coumarin-appended 1,4,7,10-tetraazacyclododecane-1,4,7-triacetate (DO3A) ligand. Dalton Transactions, 47(21), 7362-7369. doi: 10.1039/c8dt01547c. UC Berkeley: Retrieved from: http://www.escholarship.org/uc/item/0qx6776k

This journal is © The Royal Society of Chemistry. In order to reveal subtle differences between the solution chemistries of trivalent 4f and 5f elements, the physicochemical and photophysical properties of europium(iii), terbium(iii) and curium(iii)

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http://www.escholarship.org/uc/item/0qx6776k

Active actinium

Autor: Deblonde, GJP, Abergel, RJ

Publikováno v: Deblonde, GJP; & Abergel, RJ. (2016). Active actinium. Nature Chemistry, 8(11), 1084. doi: 10.1038/nchem.2653. UC Berkeley: Retrieved from: http://www.escholarship.org/uc/item/35n7n2tb

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Divalent and trivalent gas-phase coordination complexes of californium: Evaluating the stability of Cf(II)

Autor: Dau, PD, Shuh, DK, Sturzbecher-Hoehne, M, Abergel, RJ, Gibson, JK

Publikováno v: Dau, PD; Shuh, DK; Sturzbecher-Hoehne, M; Abergel, RJ; & Gibson, JK. (2016). Divalent and trivalent gas-phase coordination complexes of californium: Evaluating the stability of Cf(II). Dalton Transactions, 45(31), 12338-12345. doi: 10.1039/c6dt02414a. UC Berkeley: Retrieved from: http://www.escholarship.org/uc/item/4gj8j8h6

© 2016 The Royal Society of Chemistry. The divalent oxidation state is increasingly stable relative to the trivalent state for the later actinide elements, with californium the first actinide to exhibit divalent chemistry under moderate conditions.

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