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Publikováno v:
Journal of the American Chemical Society. 121:700-709
Enantioselective total syntheses of aloperine (1), N-methylaloperine (2), and N-allylaloperine (3) are reported. The central element of the synthetic strategy is an intramolecular Diels−Alder reaction in which the cycloaddends are tethered by a N-s
Autor:
Ping Cao, Xumu Zhang
Publikováno v:
Journal of the American Chemical Society. 121:7708-7709
Transition metal-catalyzed carbonylation reactions are fundamentally important organic transformations.1,3 Despite the great potential of asymmetric carbonylation reactions and the extensive effort devoted to this reaction during the last several dec