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Publikováno v:
JOURNAL OF THE AMERICAN CHEMICAL SOCIETY
JOURNAL OF THE AMERICAN CHEMICAL SOCIETY, 2020, 142 (35), pp.15004-15011. ⟨10.1021/jacs.0c05788⟩
JOURNAL OF THE AMERICAN CHEMICAL SOCIETY, 2020, 142 (35), pp.15004-15011. ⟨10.1021/jacs.0c05788⟩
Reduction of dinitrogen (N2) is a major challenge for chemists. Cooperation of multiple metal centers to break the strong N2 triple bond has been identified as a crucial step in both the industrial and the natural ammonia syntheses. However, reports
Publikováno v:
Journal of the American Chemical Society. 140(44)
Liquid fluoride thorium reactors have been considered as replacements for uranium-based nuclear reactors, having many economic and environmental advantages. The production of thorium is usually accompanied by the separation of thorium from rare earth
Autor:
Haiping Lin, Pingyun Feng, Min Luo, Youyong Li, Tao Wu, Jiaxu Zhang, Dongsheng Li, Wang Wei, Huajun Yang
Publikováno v:
Journal of the American Chemical Society. 140(36)
Supertetrahedral oxychalcogenide T n nanoclusters (NCs, n denotes the number of metal-chalcogen layers) integrate chemically distinct but ordered oxygen and chalcogen sites in zinc-blend-type "quantum dots". They therefore offer a new level of contro
Publikováno v:
Journal of the American Chemical Society. 140(3)
The cubic ZnS structure type and the size-dependent properties of related nanoparticles are of both fundamental and technological importance. Yet, it remains a challenge to synthesize large atom-precise clusters of this structure type. Currently, onl
Autor:
Filipp Furche, William J. Evans, Guo P. Chen, David H. Woen, Timothy J. Boyle, Joseph W. Ziller
Publikováno v:
Journal of the American Chemical Society. 139(42)
The first (N═N)2– complex of a rare-earth metal with an end-on dinitrogen bridge, {K(crypt)}2{[(R2N)3Sc]2[μ-η1:η1-N2]} (crypt = 2.2.2-cryptand, R = SiMe3), has been isolated from the reduction of Sc(NR2)3 under dinitrogen at −35 °C and char