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Publikováno v:
Inorg Chem
CoGGH, a Gly-Gly-His tripeptide coordinated to a cobalt ion, is shown to catalyze the reduction of aqueous protons to hydrogen (H(2)) in a light-driven reaction in water near neutral pH. Using [Ru(bpy)(3)](2+) as a photosensitizer and ascorbate as an
Publikováno v:
Inorganic Chemistry. 56:5519-5524
The mechanism of the dehydrogenation of N-heterocycles with the recently established bifunctional catalyst (iPrPNP)Fe(CO)(H) was investigated through experiments and density functional theory calculations (iPrPNP = iPr2PCH2CH2NCH2CH2PiPr2). In this s
Publikováno v:
Inorganic Chemistry. 55:7852-7858
A Re(I) carbonyl complex derived from 2-(2-pyridyl)-benzothiazole (pbt), [Re(H2O)(CO)3(pbt)](CF3SO3) (1), rapidly releases CO under low-power UV illumination. CO photorelease from 1 is accompanied by a change in luminescence from orange to deep blue.
Autor:
Pradip K. Mascharak, Jorge Jimenez, Annmarie Dominguez, W. M. Chamil Sameera, Jorge Martinez-Gonzalez, Indranil Chakraborty
Publikováno v:
Inorganic chemistry. 57(4)
A photoactive manganese carbonyl complex derived from dansylimidazole (Imdansyl), namely, [Mn(Imdansyl)(CO)3(phen)](CF3SO3) (1), has been synthesized and structurally characterized. This is the first luminescent manganese carbonyl-based photoCORM rep
Publikováno v:
Inorganic Chemistry. 44:6865-6878
Photoinduced charge separation is a fundamental step in photochemical energy conversion. In the design of molecularly based systems for light-to-chemical energy conversion, this step is studied through the construction of two- and three-component sys
Autor:
Indranil Chakraborty, Marilyn M. Olmstead, Pradip K. Mascharak, Samantha J. Carrington, Margarita A. Gonzalez
Publikováno v:
Inorganic chemistry. 52(19)
One monocarbonyl and one dicarbonyl complex of ruthenium(II), namely, [Ru(Cl)(CO)(qmtpm)(PPh3)]BF4 (2) and [Ru(Cl)(CO)2(qmtpm)]ClO4 (3), derived from the tridentate ligand 2-quinoline-N-(2'-methylthiophenyl)methyleneimine (qmtpm) have been synthesize
Publikováno v:
Inorganic chemistry. 44(8)
The luminescent complex Pt(dpphen)bis(arylacetylide) complex (1) (dpphen = 4,7-diphenylphenanthroline and arylacetylide = 4-ethynylbenzaldehyde) has been synthesized and characterized structurally and spectroscopically. Complex 1 has been employed in
Autor:
Chakraborty, Soma1, Wadas, Thaddeus J.1, Hester, Heidi2, Schmehl, Russell2 russ@tulane.edu, Eisenberg, Richard1 eisenberg@chem.rochester.edu
Publikováno v:
Inorganic Chemistry. 10/3/2005, Vol. 44 Issue 20, p6865-6878. 14p. 7 Diagrams, 1 Chart, 9 Graphs.