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Autor:
Khanh-Ly Claudia Nguyen, Markus Heyde, Fabian Scholten, Beatriz Roldan Cuenya, Jared P. Bruce
Publikováno v:
Angewandte Chemie (International Ed. in English)
Angewandte Chemie International Edition
Angewandte Chemie
Angewandte Chemie International Edition
Angewandte Chemie
The identification of the active sites for the electrochemical reduction of CO2 (CO2RR) to specific chemical products is elusive, owing in part to insufficient data gathered on clean and atomically well‐ordered electrode surfaces. Here, ultrahigh v
Autor:
Qin-Long Hong, Wenjing Wang, Wei Zhou, Jian Zhang, Huabin Zhang, Ping Shao, Haixia Zhang, Lirong Zheng, Luocai Yi
Publikováno v:
Angewandte Chemie. 133:16823-16828
Fundamental understanding of the dependence between the structure and composition on the electrochemical CO2 reduction reaction (CO2 RR) would guide the rational design of highly efficient and selective electrocatalysts. A major impediment to the dee
Autor:
Daniel Klose, Mikalai A. Artsiusheuski, Vitaly L. Sushkevich, Jeroen A. van Bokhoven, Gunnar Jeschke
Publikováno v:
Angewandte Chemie. 133:16080-16089
Copper-exchanged zeolites of different topologies possess high activity in the direct conversion of methane to methanol via the chemical looping approach. Despite a large number of studies, identification of the active sites, and especially their int
Autor:
Pengfei Li, Jianning Lv, Lu Dai, Bo Wang, Shuai Li, Anxiang Yin, Yanze Liu, Jiani Li, Zhejiaji Zhu
Publikováno v:
Angewandte Chemie. 133:16545-16551
2D conjugated MOFs have attracted significant interests in recent years owing to their special structural features and promising physical and chemical properties. These intriguing attributes, to a large extent, stem from the nature of incorporated li
Autor:
An, Hongyu, Wu, Longfei, Mandemaker, Laurens D B, Yang, Shuang, de Ruiter, Jim, Wijten, Jochem H J, Janssens, Joris C L, Hartman, Thomas, van der Stam, Ward, Weckhuysen, Bert M, Sub Inorganic Chemistry and Catalysis, Inorganic Chemistry and Catalysis
Publikováno v:
Angewandte Chemie-International Edition, 60(30), 16576. John Wiley and Sons Ltd
Electrocatalytic reduction of carbon dioxide (CO2) into value-added products (e.g., ethylene) is a promising approach for greenhouse gas mitigation, but many details of electrocatalytic CO2 reduction reactions (CO2RR) remain elusive. Raman spectrosco
Autor:
Kai Shao, Enlai Hu, Yu Yang, Ling Zhang, Huabin Xing, Ling Yang, Yuanjing Cui, Bin Li, Banglin Chen, Guodong Qian, Ke Jiang, Lifeng Yang, Libo Li
Publikováno v:
Angewandte Chemie. 133:16131-16138
Separation of acetylene from carbon dioxide remains a daunting challenge because of their very similar molecular sizes and physical properties. We herein report the first example of using copper(I)-alkynyl chemistry within an ultra-microporous MOF (C
Publikováno v:
Angewandte Chemie. 133:16292-16299
In recent years, copper redox mediators have attracted growing interest in dye-sensitized solar cells (DSCs). However, experiments revealed that ubiquitously used Lewis-base additives in the electrolytes coordinate to the CuII species, which restrict
Autor:
Eric J. L. McInnes, Martin Schröder, Sarah J. Day, Xue Han, Louis Kimberley, Alena M. Sheveleva, Sihai Yang, Chiu C. Tang, Xinchen Kang, Joseph H. Carter, Jiangnan Li, Gemma L. Smith, Floriana Tuna
Publikováno v:
Angewandte Chemie Int Ed
Angewandte Chemie (International Ed. in English)
Kimberley, L, Sheveleva, A M, Li, J, Carter, J H, Kang, X, Smith, G L, Han, X, Day, S J, Tang, C C, Tuna, F, Mcinnes, E J L, Yang, S & Schröder, M 2021, ' The origin of catalytic benzylic C-H oxidation over a redox-active metal-organic framework ', Angewandte Chemie International Edition . https://doi.org/10.1002/anie.202102313
Angewandte Chemie (International Ed. in English)
Kimberley, L, Sheveleva, A M, Li, J, Carter, J H, Kang, X, Smith, G L, Han, X, Day, S J, Tang, C C, Tuna, F, Mcinnes, E J L, Yang, S & Schröder, M 2021, ' The origin of catalytic benzylic C-H oxidation over a redox-active metal-organic framework ', Angewandte Chemie International Edition . https://doi.org/10.1002/anie.202102313
Selective oxidation of benzylic C−H compounds to ketones is important for the production of a wide range of fine chemicals, and is often achieved using toxic or precious metal catalysts. Herein, we report the efficient oxidation of benzylic C−H g
Autor:
Michael S. Hill, Ryan J. Schwamm, Han-Ying Liu, Nasir A. Rajabi, Claire L. McMullin, Mary F. Mahon
Publikováno v:
Angewandte Chemie (International Ed. in English)
Hill, M, Liu, H-Y D, Schwamm, R, Mahon, M, McMullin, C & Rajabi, N 2021, ' Ambiphilic Al-Cu Bonding ', Angewandte Chemie-International Edition, vol. 60, no. 26, pp. 14390-14393 . https://doi.org/10.1002/anie.202104658
Hill, M, Liu, H-Y D, Schwamm, R, Mahon, M, McMullin, C & Rajabi, N 2021, ' Ambiphilic Al-Cu Bonding ', Angewandte Chemie-International Edition, vol. 60, no. 26, pp. 14390-14393 . https://doi.org/10.1002/anie.202104658
Copper‐alumanyl complexes, [LCu‐Al(SiNDipp)], where L=carbene=NHCiPr (N,N′‐diisopropyl‐4,5‐dimethyl‐2‐ylidene) and Me2CAAC (1‐(2,6‐diisopropylphenyl)‐3,3,5,5‐tetramethyl‐pyrrolidin‐2‐ylidene) and featuring unsupported Al
Autor:
Yohann Gagné, Xavier Pannecoucke, Mathieu Frenette, Philippe Jubault, Mingbing Zhong, Taylor O. Hope, Thomas Poisson
Publikováno v:
Angewandte Chemie (International Ed. in English)
The photocatalytic hydroboration of alkenes and alkynes is reported. The use of newly‐designed copper photocatalysts with B2Pin2 permits the formation a boryl radical, which is used for hydroboration of a large panel of alkenes and alkynes. The hyd